Those aren't very impressive heat numbers for a watercooled GPU though, its not uncommon to get them down into the low 40's C with a good waterloop. This is what watercoolers call a hot loop. A hot loop has water that exceeds 10 C over the ambient temperature, while GPUs with their large silicon area don't seem to have a temperature much above the water (hence a hot loop still cools them very well) a CPU has a temperature far in excess of the water temperature.
GPU hot loops are a good way to save on radiators, so long as you don't put them in the same loop as a CPU (this guy didn't). My estimate would be the water is somewhere around +25C, which is likely accelerating damage to the pump and the tubing greatly, but it'll work for a while before the heat slowly but surely destroys the parts.
You're expecting custom-loop results from a closed loop? Okay...