The FX60 is the fastest, I think. But they are rather expensive. If I was upgrading the CPU, and couldn't do a whole platform upgrade, I would look at Opteron 165's and 170's. Dual core, full 1MB L2 per core, and they overclock very well if your motherboard can handle the 9x multiplier of the 165 (the 10x multiplier of the 170 will likely allow for higher clocks, though).
Both CPU's are fairly cheap on Ebay, $20-$30. I would do this over an FX chip, no way I'd spend that much money on an older platform.