I'm still really digging the Lillywhite Sessions--favorites from that disc are Gray Street, Bartender, JTR, and my utter favorite--Big Eyed Fish (if you have not heard this song go thee hence and download!).
From his other releases:
Best of What's Around
Seek Up
The Song That Jane Likes
All Along The Watchtower (it's his best cover by far)
Dancing Nancies
Tripping Billies
#41 (my fav. DMB tune of all time)
Crush
Dreaming Tree
Spoon
If I Had It All
Mother Father
There's really not a DMB song I don't like though.
l2c