Well, you could get a 6600GT for around $130~$150, but in general it is better to buy a single, more powerful card than to go SLI. From AT's recent 6800GS article:
"We also generally do not recommend SLI as an upgrade option. The main benefit of multi-GPU technology these days is to increase the maximum performance beyond the fastest single card on the market. ATI and NVIDIA have kept upgrade cycles fairly consistent over the past few years. It makes sense to spend money on a card that will bring increased performance and more features to a system when a new generation of GPU comes out rather than augmenting an aging card with another of the same type."