Windows NT as in NT 4.0 because XP and Vista are based around the NT core. I'm guessing that you're talking about 4.0 and I highly doubt that you could get PCI-E to work properly (if at all) underneath the platform as I'm sure that there aren't any drivers available. Why on earth would you want to try anyways?
Please stop using WindowsNT to refer to NT 4 as if it's the only release of NT, if you look you'll see that XP is NT 5.1 and Vista is 6.0.
But NT 4 isn't supported any more so you really should follow drag's advice and only run it under some form of virtualization if you really need it these days.
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