Hey Evilsponge, having two sticks of RAM will increase your performance slightly, like mboy said, but it won't help your overclock. Because of the added latency addressing two sticks of RAM, you may actually have to lower your memory timings to get two sticks to run at the same speed as one. Running in dual-channel means that the chipset has the ability to combine the bandwidth of both sticks of RAM when delivering information to the CPU. Unfortunately, the AMD Athlon, Durun, XP are designed to use the bandwidth of one channel of DDR, so dual-channel doesn't help all that much, but every little bit helps right?
Mboy, I don't agree with you that the nForce is that much faster than the other chipsets, especially the KT400A that is soon to be released. Preliminary tests I have seen show the KT400A to beat out even the nForce2 in dual-channel mode. Also, I had zero problems with my previous AMD boxes with the KT266A and KT333 chipsets, so I am not sure as to what you are talking about being buggy. And I was able to take them up over 210 FSB, something I haven't seen someone claim with an nForce2, so any small performace gain on the part of the nForce 2 would be lost due to lower max FSB. Don't get me wrong, I like the nForce 2, but VIA makes fine chipsets too, and until recently, they made by far the best AMD chipsets, so it is good they have some competition.
Evilsponge, have you hit the limit of your CPU yet? You may wanna try lowering your FSB a bit a raising your multiplier and CPU voltage a bit. Higher FSB will give you a nice performance boost, but nothing beats more raw CPU power. As others have said, you can raise the vcore a little more and still be safe. Also, keep in mind that the higher FSB is not only harder on your RAM, but on your CPU. For example, it will take more juice to run your CPU at 2.xx GHz at 200 FSB than to run it at the same speed at 133 FSB, so keep that in mind when overclocking. A couple years ago when I had a 1 GHz Athlon, I left the FSB at 133 and took the multiplier up until the chip wouldn't go anymore, around 1.4 GHz as I recall. Then I started lowering the multiplier while running up the FSB to keep my speed to find the sweet spot. AMD chips are fun to overclock since the multiplier is unlocked.