mikef208,
I can't comment on the VCRAM cause I don't know jack about that, but as far as the memory speed for the kt133a chipset, the mhz stays the same. The only change they made was enabling 133mhz fsb for the cpu. Overclocking will yield mhz of the fsb and memory in tandem(145mhz fsb =145mhz RAM) although thats not truly the case because the fsb is ddr so it would be 290mhz fsb = 145mhz RAM. I'm not sure if you can change the settings for fsb separate from the memory(i.e., set the fsb to 145 and leave the RAM at 133). I know on the kt133 chipset, the memory was 133 while the fsb was 100 and that was the selling point of the kt133 that it could run the memory asynchronously from the fsb so you could use pc133 ram. Anyway, the bottom line is that on the kt133a boards, if the fsb is set to 133, the memory will be set to 133(unless you can tweek that in the bios) and you can walk those two up together when overclocking.
As far as ram is concerned, I have some mushkin rev3 which is rated cas2 at 150 and thats also another important point when overclocking. You'll get better results being able to run at cas 2. I read an article(if I find it I'll post it on this thread for you) that in order to get the same performance out of cas 3, you'd have to run it something like 15mhz higer than the cas2. So it seems that if your going to try for some serious overclock, you'd want the memory to handle cas 2 at the higher speeds. If anything I've posted here is inaccurate or needs some better explanation, please jump in and correct it. We're all here to learn from each other.
Taplight