Howdy there Space Cowboy! Your kinda going at it backwards, you should be cranking up the HTT(FSB) and only increasing the voltages when you have to. Your ram volts are way to high for that ram.
With the ram that you have, and the fact that you have 2GB its not going to overclock well at all. But thats fine because high ramspeed means squat on A64's unless your a benchmarking fanatic.
Drop the DDRvolts back to 2.75 and find the memory dividers on your board and set to 166, this will run your ram at a lower speed than the HTT. Leave the vcore at 1.55, Set the HTT multi(also known as LDT) to 4x, Set HTT(FSB) to 220mhz, CPUmulti 11x. It should boot up no problem with those settings at 2420mhz, then increase the HTT 3-5mhz at a time and test for stability as you go with Prime95 or SuperPI (free downloads). Once you start getting errors in Prime or PI, then back down to your previous setting and run Prime for several hours (preferably overnight), if you get errors back it down a few more mhz, and try again. Once it will run prime overnight you know its a good overclock and won't give you any problems. I'm guessing you can get in the 2.6-2.65 range with that chip, just check you CPU temps after a couple of hours of Prime and as long as they are less than 65c your OK. With that DFI board you can push it farther with more vcore, but personally I wouldn't go above 1.60 without watercooling or phase change.