CSRSS = client server runtime sub-system, and is the primary component of the Windows subsystem on NT. It is a critical system process, and it is absolutely not to blame here.
Rundll32.exe is a Microsoft-supplied wrapper application that can be invoked by ANY other program or driver on your system. Many applications REQUIRE this application to function properly, so you cannot delete it! Its entire purpose in life is to load a specified DLL (specified by a command-line argument) and then to invoke a function exported by that DLL.
rundll32.exe is commonly used to force code to run in a separate process, for example if you want to run a 3rd party extension or custom task/plugin but you don't trust the plugin enough to run it in your own address space. (Usually if you load a DLL into your process address space and it crashes, then your process will die. Running the code via rundll32.exe will create a 2nd process that is isolated and cannot crash your process.)
The crash you are seeing is
NOT caused by Rundll32.exe, but rather is caused by the DLL which rundll32.exe loads. To track down the culprit, you must find the provider of this DLL and possibly who is invoking it.
There are two pieces of information I would use to track it down, both of which require the process object to be alive for inspection (when you get the "Such and such program has encountered an error" dialog, the process is usually gone). To keep the process alive for inspection after crashing, I would install a post-mortem debugger like WinDBG (available for free from Microsoft).
Then, the next time you see the rundll32.exe crash, you can look for two things which can help point to a culprit:
1) Which process spawned the rundll32.exe PID? Process explorer or tlist.exe can show you the process hierarchy. Knowing the identity of the parent process will help you understand why rundll32.exe is running, or at least its context.
2) What are the command-line arguments to rundll32.exe? One of the command-line arguments is the pathname for the DLL that crashed (see
this Microsoft KB). The author of the DLL is the likely culprit.