BossDog: The Promise FastTrak66 can use up to 4 hard drives. And ONLY hard drives, your motherboard controller has to do any other devices you want.
Mister T:
For performance 4x15GB 7200RPM RAID0 would be the best.
Adding drives to a RAID0 isn't linear performance increase though (that is to say 2 drives aren't twice as fast as one, 3 drives aren't 3 times as fast as 1 and so on) because all the drives have to seek, you can't improve seek times with a RAID. 2x RAID0 is probably the best for price to performance. Wait wtf am I talking about

This is RAID, no price/performance pansies here hehehe.
Yes 4 drives will be better than 2. Watch out though, I read somewhere that the max RAID Array size in Win98 (for the Promise card) is 64GB (not that this matters with 4x15 drives, just a general warnning).
There are lots of exotic RAID schemes, by far the most common are RAID1 and RAID0 though, RAID1 duplicates data and increases read performance (you have two copies to read from), but tends to hinder write performance (you have to write to both drives).
RAID0 is what you want for performance, this reads/writes alternating chunks to each drive and boosts performance quite nicely*. Of course if one drive in the Array crashes, everything on the whole Array is lost.
Take it easy.
*: (Fine details if you want them) The only thing that is actually improved is the data transfer speed, so for large files RAID0 will show huge improvements, however the seek speed does not improve on a RAID because all the drives have to seek together (the same length of time as single drive seek). So if you are dealing with lots of files strewn all over the drive a RAID0 array won't perform much better than a single drive.
However, since most disk activity while running programs is virtual memory, if you set up your swap file so it's continuous on the disk (well the array, but it looks like a single disk once set up) this will minimize the amount of seeking that needs to be done, so you should get a respectable performance boost out of a RAID0 set up.