technically you could run the two drives in raid 0, but they way striping works, you would only have 72gb of usable space
(capacity of smalles drive) x (number of drives)
raid 0 is pure striping, where bits are alternatly written to 2 or more drives
raid 1 is mirroring, where data is constantly mirrored so you always have a perfect backup
raid 0+1 is a combination, which requires 4 or more drives...basically 2 sets of striped drives mirrored
after that i'm not so sure...
but for your current setup raid 0 wouldn't be a good idea cause you'd be losing a whole lot of space
also, its usually a good idea to use drives of identical speed when striping, otherwise you might have latency issues while the controller waits for data to be written to the slower drive.
hope that helps
S-ata or ide doesn't really matter yet...but if you're buying a raid controller you might want s-ata to be future proof.
-Vivan