The episode called Time Enough at Last. Reminds me of what I would do with my PC game collection.
First, Rod Sterling was a frikken genius. His ability to write such a diversity of episodes on such a short schedule was amazing. However, I was less thrilled when he dealt with political topics because those episodes seem much more dated.
Favorite episode is easily 'Nick of Time'. William Shatner was perfect for many of those scripts.