Zebo's OCing guide is your friend 🙂 Seriously, all the info needed for OCing is in there.
First determine your max HTT [akin to FSB] speed.
Set your CPU multi to maybe 6x or even 5x, & see how high you can get your HTT before it starts to get unstable.
Always make sure your LDTxHTT = 1000 or less.
To make it easy while testing, just leave it at 3x, since it's very unlikely you'll get the HTT higher than 333 anyway (which would be 3x333=999)
I would worry about RAM speed last, so set the RAM to the lowest divider (100 aka 2:1) with very loose timings.
Check that the AGP/PCI is locked (should be a bios setting somewhere)
If that mobo has four SATA ports & you are using one, you may have to find out which ones are locked & which are not. Usually the non-nForce ports are the locked ones.
For CPU stability testing, use Prime95 Torture Test small FFTs.
Good luck!