Depends on what kind of RAM you have. If you have DDR 400, or some good DDR 333 sticks, leaving those settings on Auto will be fine. You should set the AGP frequency to 66 and the PCI to 33.
However, all of the DDR 333 sticks I've every owned could not overclock past 166 very much. I hope you have some decent RAM. It is not adviseable to run a memory divider with Socket A processors, or at least it was not adviseable with Athlon XPs. Even if you were able to overclock the processor much farther by using a memory divider, performance could actually get worse.
I'd also like to say good luck with the overclock. I tried to clock a Sempron 2500+ on an Abit NF7-S2 and it would fail to post no matter how little I upped the FSB or how much voltage I applied. I blame the crap motherboard for this problem, though, because itss overclocking options are very basic.