Murph, there is not much advantage to running the memory at 1066, since you are not synchronous with the cpu. At a bus of 1333, your memory is running at 5:4. Not really a good idea, since the core2 is much less efficient at these memory splits. I tried it and got lower 3dmark06 scores. I have some DDR2-1066 (corsair) around, and it did not help. The only advantage is if you are running 1066 fsb, and keep the memory at 1:1, then it screams. However I have not been able to overclock as well at the 1066 fsb (4 x266). I seem to get the most success with a 320-333 x 4 fsb, and then adjusting the multi. Right now I am at 3.66, fsb 333 x 4, multi at 11, memory at 667 which is 2:1. The core2 seems to like 1:1 and 2:1 memory splits, it is the way it was designed. If you are trying for maximum overclock, just back down and increase the cpu speed. You will get much more performance that way. I have been playing with an E6400 and high fsbs, and the same thing. Running an E6400 at fixed multi of 8, fsb up to 1333 (from 1066), raised cpu from 2.13 to 2.66, memory at 999 (1000) and it is stable but some programs do not run, when adjusted to 667, flawless. And the corsair memory needs to run at 2.1V (2.2V if ddr2 1000), for the highest timings. Keep the timings tight, but drop the speed to 667.
Noushy