Nope. You need an iEvolution for it to work at all, and even then the situation is not good. New firmware broke that cart months ago, and for some reason Team Cyclops seems to have dropped off the face of the Earth. You'll want to look for another flash cart if you need one for a 3DS.
I don't have a 3DS, so I can't give you any firsthand recommendations. I'd suggest looking around gbatemp (including the forums) before making any purchasing decisions.
For what it's worth, I don't use flash cards for piracy, though I know I'm in the minority.
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