The extended test of the 2TB ELEMENTS USB HD finished this morning. It passed. No other info was provided, I poked around looking for specifics, data, indications of whether or not bad sectors were discovered, whatever but couldn't find any more info in WDDLD. Ah... I just brought up the SMART disk info. There are 6 X's, the rest checks. I don't know how to interpret the info. Crystaldiskinfo calls the disk "Good."
I still can't delete the temp files that alerted me to an issue, that stopped Windows Copy command from completing.
Perhaps (

) some data is now in better shape? I have no way of knowing, no reason to think so, but maybe it is. I can copy data back to the NAS from the just _scanned_ USB HD, this time using something more helpful than the Copy command. What do you think?
Edit: I suppose I should do as you suggest and test the NAS's HDs, presumably by running the WDLDIAG extended test on them? That appears to not provide feedback other than PASSED or not passed, right?
Are there other diagnostic techniques that would be better used here?
Edit2: I'm considering copying everything on the USB drive (there's only around 360GB total on the USB HD) to a different USB drive, I have several, before defragmenting. I suppose it would be an extra step that would decrease the chances of losing anything. In copying (or robocopying or whatever) I imagine that the data will be automatically defragmented as placed on the copied-to HD. I'd have an extra version of the data in case something goes wrong. All this likely before testing the NAS HDs.