You might want to wait for a chemist to reply, but I'd expect CLR to turn rust a color like dark, not just make it vanish. I'd first try scrubbing with a stiff brush and detergent, then power washing if that wasn't enough, but suspect that the effort to remove most of the rust, will leave the remaining surface looking different than the surrounding area.
One thing you could try is putting some in a tiny spot to see what happens instead of treating the whole area.