You can. Wouldn't make much sense, though since afaik the faster card is "downgraded" to fit the slower card.
My issue with crossfire is that the profiles for the most part come out after the game. Despite AMD splitting the crossfire profiles from the driver package they often lag the drivers and lag weeks after a games release, and sometimes we are waiting months for the release. However almost all games just need a profile rather than a patch in the drivers to work well with crossfire. So you if you set it up yourself it more than often works until AMD release the official profile (which normally just contains the same setup you came upon as well).
Now that isn't to say NVidia's SLI support system isn't by default better, I think it often is. But a large part of that seems to be they are ahead of the curve with the releases so the games have support when they are released, which is the way round it should be. But I don't think there is a universal truth that AMD's crossfire is bad and NVidia's is good, they both have problems which you can see in forums all over the place.